[S,S]-Ethylene diamine disuccinic acid; Notice of Filing a Pesticide Petition to Establish a Tolerance for a Certain Pesticide Chemical in or on Food, 3026-3032 [05-824]
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Federal Register / Vol. 70, No. 12 / Wednesday, January 19, 2005 / Notices
included in the public docket and EPA’s
electronic public docket without prior
notice. If you have any questions about
CBI or the procedures for claiming CBI,
please consult the person listed under
FOR FURTHER INFORMATION CONTACT.
E. What Should I Consider as I Prepare
My Comments for EPA?
You may find the following
suggestions helpful for preparing your
comments:
1. Explain your views as clearly as
possible.
2. Describe any assumptions that you
used.
3. Provide any technical information
and/or data you used that support your
views.
4. If you estimate potential burden or
costs, explain how you arrived at your
estimate.
5. Provide specific examples to
illustrate your concerns.
6. Offer alternatives.
7. Make sure to submit your
comments by the comment period
deadline identified.
8. To ensure proper receipt by EPA,
identify the appropriate docket ID
number in the subject line on the first
page of your response. It would also be
helpful if you provided the name, date,
and Federal Register citation related to
your comments.
II. Background
A. What Action is the Agency Taking?
Under section 4 of the Federal
Insecticide, Fungicide, and Rodenticide
Act (FIFRA), EPA is reevaluating
existing pesticides to ensure that they
meet current scientific and regulatory
standards. Using a modified,
streamlined version of its public
participation process, EPA has
completed a RED for the low risk
pesticide, nitrogen under section
4(g)(2)(A) of FIFRA. EPA has
determined that the data base to support
reregistration is substantially complete
and that products containing nitrogen
will be eligible for reregistration,
provided the risks are mitigated either
in the manner described in the RED or
by another means that achieves
equivalent risk reduction. Upon
submission of any required product
specific data under section 4(g)(2)(B)
and any necessary changes to the
registration and labeling (either to
address any concerns identified in the
RED or as a result of product specific
data), EPA will make a final
reregistration decision under section
4(g)(2)(C) for products containing
nitrogen.
Nitrogen is used commercially to
generate an inert atmosphere usually for
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product packaging. In the food industry,
it is used to preserve packaged foods,
such as ground coffee, by displacing
oxygen. As a pesticide active ingredient,
nitrogen may be used as a fumigant to
control insects in structures and on
stored food commodities. Currently
there is only one registered end-use
product containing nitrogen as the
active ingredient. As a pesticide inert it
is used as an aerosol propellant.
EPA must review tolerances and
tolerance exemptions that were in effect
when the Food Quality Protection Act
(FQPA) was enacted in August 1996, to
ensure that these existing pesticide
residue limits for food and feed
commodities meet the safety standard
established by the new law. Tolerances
are considered reassessed once the
safety finding has been made or a
revocation occurs. EPA has reviewed
and made the requisite safety finding for
the nitrogen tolerances included in this
notice.
EPA is applying the principles of
public participation to all pesticides
undergoing reregistration and tolerance
reassessment. The Agency’s Pesticide
Tolerance Reassessment and
Reregistration; Public Participation
Process, published in the Federal
Register on May 14, 2004, explains that
in conducting these programs, the
Agency is tailoring its public
participation process to be
commensurate with the level of risk,
extent of use, complexity of issues, and
degree of public concern associated
with each pesticide. EPA can
expeditiously reach decisions for
pesticides like nitrogen, which pose no
risk concerns, have low use, affect few
if any stakeholders, and require little/no
risk mitigation. Once EPA assesses uses
and risks for such pesticides, the
Agency may go directly to a decision
and prepare a document summarizing
its findings. The Agency therefore is
issuing the low risk nitrogen RED, risk
assessments, and related documents
simultaneously for public comment.
The reregistration program is being
conducted under Congressionally
mandated time frames, and EPA
recognizes the need both to make timely
decisions and to involve the public in
finding ways to effectively mitigate
pesticide risks. Nitrogen, however,
poses no risks that require mitigation.
The Agency therefore is issuing the
nitrogen RED, its risk assessments, and
related support materials
simultaneously for public comment.
The comment period is intended to
provide an opportunity for public input
and a mechanism for initiating any
necessary amendments to the RED. All
comments should be submitted using
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the methods in Unit I. of the
SUPPLEMENTARY INFORMATION,
and must
be received by EPA on or before the
closing date. These comments will
become part of the Agency Docket for
nitrogen. Comments received after the
close of the comment period will be
marked ‘‘late.’’ EPA is not required to
consider these late comments.
EPA will carefully consider all
comments received by the closing date
and will provide a Response to
Comments Memorandum in the Docket
and electronic Edocket. If any comment
significantly affects the document, EPA
also will publish an amendment to the
RED in the Federal Register. In the
absence of substantive comments
requiring changes, the nitrogen RED will
be implemented as it is now presented.
B. What is the Agency’s Authority for
Taking this Action?
Section 4(g)(2) of FIFRA as amended
directs that, after submission of all data
concerning a pesticide active ingredient,
‘‘the Administrator shall determine
whether pesticides containing such
active ingredient are eligible for
reregistration,’’ before calling in product
specific data on individual end-use
products and either reregistering
products or taking other ‘‘appropriate
regulatory action.’’
Section 408(q) of the Federal Food,
Drug, and Cosmetic Act (FFDCA), 21
U.S.C. 346a(q), requires EPA to review
tolerances and exemptions for pesticide
residues in effect as of August 2, 1996,
to determine whether the tolerance or
exemption meets the requirements of
section 408(b)(2) or (c)(2) of FFDCA.
This review is to be completed by
August 3, 2006.
List of Subjects
Environmental protection, Pesticides
and pests.
Dated: December 17, 2004.
Debra Edwards,
Director, Special Review and Reregistration
Division, Office of Pesticide Programs.
[FR Doc. 05–1025 Filed 1–18–05; 8:45 am]
BILLING CODE 6560–50–S
ENVIRONMENTAL PROTECTION
AGENCY
[OPP–2004–0297; FRL–7690–5]
[S,S]-Ethylene diamine disuccinic acid;
Notice of Filing a Pesticide Petition to
Establish a Tolerance for a Certain
Pesticide Chemical in or on Food
Environmental Protection
Agency (EPA).
AGENCY:
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Federal Register / Vol. 70, No. 12 / Wednesday, January 19, 2005 / Notices
ACTION:
Notice.
SUMMARY: This notice announces the
initial filing of a pesticide petition
proposing the establishment of
regulations for residues of a certain
pesticide chemical in or on various food
commodities.
DATES: Comments, identified by docket
identification (ID) number OPP–2004–
0297, must be received on or before
February 18, 2005.
ADDRESSES: Comments may be
submitted electronically, by mail, or
through hand delivery/courier. Follow
the detailed instructions as provided in
Unit I. of the SUPPLEMENTARY
INFORMATION.
FOR FURTHER INFORMATION CONTACT:
Bipin Gandhi, Registration Division
(7505C), Office of Pesticide Programs,
Environmental Protection Agency, 1200
Pennsylvania Ave., NW., Washington,
DC 20460–0001; telephone number:
(703) 308–8380; e-mail address:
gandhi.bipin@epa.gov.
SUPPLEMENTARY INFORMATION:
I. General Information
A. Does this Action Apply to Me?
You may be potentially affected by
this action if you are an agricultural
producer, food manufacturer, or
pesticide manufacturer. Potentially
affected entities may include, but are
not limited to:
• Crop production (NAICS 111)
• Animal production (NAICS 112)
• Food manufacturing (NAICS 311)
• Pesticide manufacturing (NAICS
32532)
This listing is not intended to be
exhaustive, but rather provides a guide
for readers regarding entities likely to be
affected by this action. Other types of
entities not listed in this unit could also
be affected. The North American
Industrial Classification System
(NAICS) codes have been provided to
assist you and others in determining
whether this action might apply to
certain entities. If you have any
questions regarding the applicability of
this action to a particular entity, consult
the person listed under FOR FURTHER
INFORMATION CONTACT.
B. How Can I Get Copies of this
Document and Other Related
Information?
1. Docket. EPA has established an
official public docket for this action
under docket ID number OPP–2004–
0297. The official public docket consists
of the documents specifically referenced
in this action, any public comments
received, and other information related
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to this action. Although a part of the
official docket, the public docket does
not include Confidential Business
Information (CBI) or other information
whose disclosure is restricted by statute.
The official public docket is the
collection of materials that is available
for public viewing at the Public
Information and Records Integrity
Branch (PIRIB), Rm. 119, Crystal Mall
#2, 1801 S. Bell St., Arlington, VA. This
docket facility is open from 8:30 a.m. to
4 p.m., Monday through Friday,
excluding legal holidays. The docket
telephone number is (703) 305–5805.
2. Electronic access. You may access
this Federal Register document
electronically through the EPA Internet
under the ‘‘Federal Register’’ listings at
https://www.epa.gov/fedrgstr/.
An electronic version of the public
docket is available through EPA’s
electronic public docket and comment
system, EPA Dockets. You may use EPA
Dockets at https://www.epa.gov/edocket/
to submit or view public comments,
access the index listing of the contents
of the official public docket, and to
access those documents in the public
docket that are available electronically.
Although not all docket materials may
be available electronically, you may still
access any of the publicly available
docket materials through the docket
facility identified in Unit I.B.1. Once in
the system, select ‘‘search,’’ then key in
the appropriate docket ID number.
Certain types of information will not
be placed in the EPA Dockets.
Information claimed as CBI and other
information whose disclosure is
restricted by statute, which is not
included in the official public docket,
will not be available for public viewing
in EPA’s electronic public docket. EPA’s
policy is that copyrighted material will
not be placed in EPA’s electronic public
docket but will be available only in
printed, paper form in the official public
docket. To the extent feasible, publicly
available docket materials will be made
available in EPA’s electronic public
docket. When a document is selected
from the index list in EPA Dockets, the
system will identify whether the
document is available for viewing in
EPA’s electronic public docket.
Although not all docket materials may
be available electronically, you may still
access any of the publicly available
docket materials through the docket
facility identified in Unit I.B. EPA
intends to work towards providing
electronic access to all of the publicly
available docket materials through
EPA’s electronic public docket.
For public commenters, it is
important to note that EPA’s policy is
that public comments, whether
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submitted electronically or in paper,
will be made available for public
viewing in EPA’s electronic public
docket as EPA receives them and
without change, unless the comment
contains copyrighted material, CBI, or
other information whose disclosure is
restricted by statute. When EPA
identifies a comment containing
copyrighted material, EPA will provide
a reference to that material in the
version of the comment that is placed in
EPA’s electronic public docket. The
entire printed comment, including the
copyrighted material, will be available
in the public docket.
Public comments submitted on
computer disks that are mailed or
delivered to the docket will be
transferred to EPA’s electronic public
docket. Public comments that are
mailed or delivered to the docket will be
scanned and placed in EPA’s electronic
public docket. Where practical, physical
objects will be photographed, and the
photograph will be placed in EPA’s
electronic public docket along with a
brief description written by the docket
staff.
C. How and to Whom Do I Submit
Comments?
You may submit comments
electronically, by mail, or through hand
delivery/courier. To ensure proper
receipt by EPA, identify the appropriate
docket ID number in the subject line on
the first page of your comment. Please
ensure that your comments are
submitted within the specified comment
period. Comments received after the
close of the comment period will be
marked ‘‘late.’’ EPA is not required to
consider these late comments. If you
wish to submit CBI or information that
is otherwise protected by statute, please
follow the instructions in Unit I.D. Do
not use EPA Dockets or e-mail to submit
CBI or information protected by statute.
1. Electronically. If you submit an
electronic comment as prescribed in this
unit, EPA recommends that you include
your name, mailing address, and an email address or other contact
information in the body of your
comment. Also include this contact
information on the outside of any disk
or CD ROM you submit, and in any
cover letter accompanying the disk or
CD ROM. This ensures that you can be
identified as the submitter of the
comment and allows EPA to contact you
in case EPA cannot read your comment
due to technical difficulties or needs
further information on the substance of
your comment. EPA’s policy is that EPA
will not edit your comment, and any
identifying or contact information
provided in the body of a comment will
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Federal Register / Vol. 70, No. 12 / Wednesday, January 19, 2005 / Notices
be included as part of the comment that
is placed in the official public docket,
and made available in EPA’s electronic
public docket. If EPA cannot read your
comment due to technical difficulties
and cannot contact you for clarification,
EPA may not be able to consider your
comment.
i. EPA Dockets. Your use of EPA’s
electronic public docket to submit
comments to EPA electronically is
EPA’s preferred method for receiving
comments. Go directly to EPA Dockets
at https://www.epa.gov/edocket/, and
follow the online instructions for
submitting comments. Once in the
system, select ‘‘search,’’ and then key in
docket ID number OPP–2004–0297. The
system is an ‘‘anonymous access’’
system, which means EPA will not
know your identity, e-mail address, or
other contact information unless you
provide it in the body of your comment.
ii. E-mail. Comments may be sent by
e-mail to opp-docket@epa.gov,
Attention: Docket ID Number OPP–
2004–0297. In contrast to EPA’s
electronic public docket, EPA’s e-mail
system is not an ‘‘anonymous access’’
system. If you send an e-mail comment
directly to the docket without going
through EPA’s electronic public docket,
EPA’s e-mail system automatically
captures your e-mail address. E-mail
addresses that are automatically
captured by EPA’s e-mail system are
included as part of the comment that is
placed in the official public docket, and
made available in EPA’s electronic
public docket.
iii. Disk or CD ROM. You may submit
comments on a disk or CD ROM that
you mail to the mailing address
identified in Unit I.C.2. These electronic
submissions will be accepted in
WordPerfect or ASCII file format. Avoid
the use of special characters and any
form of encryption.
2. By mail. Send your comments to:
Public Information and Records
Integrity Branch (PIRIB) (7502C), Office
of Pesticide Programs (OPP),
Environmental Protection Agency, 1200
Pennsylvania Ave., NW., Washington,
DC 20460–0001, Attention: Docket ID
Number OPP–2004–0297.
3. By hand delivery or courier. Deliver
your comments to: Public Information
and Records Integrity Branch (PIRIB),
Office of Pesticide Programs (OPP),
Environmental Protection Agency, Rm.
119, Crystal Mall #2, 1801 S. Bell St.,
Arlington, VA, Attention: Docket ID
Number OPP–2004–0297. Such
deliveries are only accepted during the
docket’s normal hours of operation as
identified in Unit I.B.1.
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D. How Should I Submit CBI to the
Agency?
Do not submit information that you
consider to be CBI electronically
through EPA’s electronic public docket
or by e-mail. You may claim
information that you submit to EPA as
CBI by marking any part or all of that
information as CBI (if you submit CBI
on disk or CD ROM, mark the outside
of the disk or CD ROM as CBI and then
identify electronically within the disk or
CD ROM the specific information that is
CBI). Information so marked will not be
disclosed except in accordance with
procedures set forth in 40 CFR part 2.
In addition to one complete version of
the comment that includes any
information claimed as CBI, a copy of
the comment that does not contain the
information claimed as CBI must be
submitted for inclusion in the public
docket and EPA’s electronic public
docket. If you submit the copy that does
not contain CBI on disk or CD ROM,
mark the outside of the disk or CD ROM
clearly that it does not contain CBI.
Information not marked as CBI will be
included in the public docket and EPA’s
electronic public docket without prior
notice. If you have any questions about
CBI or the procedures for claiming CBI,
please consult the person listed under
FOR FURTHER INFORMATION CONTACT.
E. What Should I Consider as I Prepare
My Comments for EPA?
You may find the following
suggestions helpful for preparing your
comments:
1. Explain your views as clearly as
possible.
2. Describe any assumptions that you
used.
3. Provide copies of any technical
information and/or data you used that
support your views.
4. If you estimate potential burden or
costs, explain how you arrived at the
estimate that you provide.
5. Provide specific examples to
illustrate your concerns.
6. Make sure to submit your
comments by the deadline in this
notice.
7. To ensure proper receipt by EPA,
be sure to identify the docket ID number
assigned to this action in the subject
line on the first page of your response.
You may also provide the name, date,
and Federal Register citation.
II. What Action is the Agency Taking?
EPA has received a pesticide petition
as follows proposing the establishment
and/or amendment of regulations for
residues of a certain pesticide chemical
in or on various food commodities
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under section 408 of the Federal Food,
Drug, and Cosmetic Act (FFDCA), 21
U.S.C. 346a. EPA has determined that
this petition contains data or
information regarding the elements set
forth in FFDCA section 408(d)(2);
however, EPA has not fully evaluated
the sufficiency of the submitted data at
this time or whether the data support
granting of the petition. Additional data
may be needed before EPA rules on the
petition.
List of Subjects
Environmental protection,
Agricultural commodities, Feed
additives, Food additives, Pesticides
and pests, Reporting and recordkeeping
requirements.
Dated: December 29, 2004.
Betty Shackleford,
Acting Director, Registration Division, Office
of Pesticide Programs.
Summary of Petition
The petitioner summary of the
pesticide petition is printed below as
required by FFDCA section 408(d)(3).
The summary of the petition was
prepared by the petitioner and
represents the view of the petitioner.
The summary may have been edited by
EPA if the terminology used was
unclear, the summary contained
extraneous material, or the summary
unintentionally made the reader
conclude that the findings reflected
EPA’s position and not the position of
the petitioner. The petition summary
announces the availability of a
description of the analytical methods
available to EPA for the detection and
measurement of the pesticide chemical
residues or an explanation of why no
such method is needed.
The Associated Octel Company,
Limited
PP 4E6818
EPA has received a pesticide petition
(4E6818) from The Associated Octel
Company, Limited, P.O. Box 17, Oil
Sites Road, Ellesmere Port, South Wirral
L65 4HF, United Kingdom proposing,
pursuant to section 408(d) of the
FFDCA, 21 U.S.C. 346a(d), to amend 40
CFR part 180 to establish an exemption
from the requirement of a tolerance for
[S,S]-ethylene diamine disuccinic acid,
CAS Reg. No. 20846–91–7. EPA has
determined that the petition contains
data or information regarding the
elements set forth in section 408(d)(2) of
the FFDCA; however, EPA has not fully
evaluated the sufficiency of the
submitted data at this time or whether
the data support granting of the petition.
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Additional data may be needed before
EPA rules on the petition.
A. Residue Chemistry
1. Plant metabolism. [S,S]-Ethylene
diamine disuccinic acid is a chelating
agent that is used as a vehicle to deliver
micronutrients essential for healthy and
rapid growth, such as iron and cobalt,
to plants. It is unknown whether or not
plants would uptake [S,S]-ethylene
diamine disuccinic acid that might
leach into the soil when applied as a
minor component of pesticide
formulations. However, organic
chelating agents are not absorbed
normally by growing plants. It appears
that the primary role the chelate plays
is to hold the metallic cations near the
root surface until direct absorption of
the free cation can take place. Once the
micronutrient cations are inside the
plant, other organic chelates (such as
citrates) may be carriers of these cations
to different parts of the plant (Ref. 1).
Therefore, it is unlikely that [S,S]ethylene diamine disuccinic acid would
accumulate within plant tissue through
its application to the soil as a minor
component of pesticide formulations.
2. Analytical method. An analytical
method has not been proposed because
[S,S]-ethylene diamine disuccinic acid
residues harmful to plants and animals
are highly unlikely to occur when it is
applied as part of the proposed
pesticide formulation and according to
that formulation’s label directions for
use.
3. Magnitude of residues. A waiver of
the residue data has been requested
because [S,S]-ethylene diamine
disuccinic acid is produced by
actinomycetes, Amycolatopis japonica
sp. nov. (Ref. 2) and Amycolatopsis
orientalis (Ref. 3), which are naturally
occurring bacteria, degrades rapidly and
is completely mineralized in the soil,
will have limited accessibility to plants
in the proposed use pattern, and
exhibits low mammalian toxicity. [S,S]Ethylene diamine disuccinic acid is a
siderophore produced by actinomycetes,
and it functions symbiotically with
plants to assist in the transport of soil
metals to plant rootlets. The use of [S,S]ethylene diamine disuccinic acid,
therefore, does not constitute the
addition of a foreign material to the soil;
rather, it is a compound that soil
microorganisms and plants already
encounter. Natural mechanisms already
exist for the degradation and/or
utilization of [S,S]-ethylene diamine
disuccinic acid in the soil/plant
microsystem. Moreover, organic
chelates are not absorbed normally by
growing plants, and residues are not
expected in plants.
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B. Toxicological Profile
1. Acute toxicity. The acute toxicity of
[S,S]-ethylene diamine disuccinic acid
was studied in several studies using
male and female rats via the oral,
dermal, and inhalation routes. In two
acute oral toxicity studies, the lethal
dose (LD)50 for both males and females
was established at >2,700 milligrams/
kilogram body weight (mg/kg bwt) and
>2,000 mg/kg bwt, respectively, which
were the highest dose levels tested. For
the two acute dermal toxicity studies,
the LD50 for both males and females was
established at >2,640 mg/kg bwt and >
2,000 mg/kg bwt, respectively, which
were the highest dose levels tested. For
the acute inhalation study, the lethal
concentration (LC)50 was established at
>1.49 milligrams/liter (mg/L), which
was the highest concentration that could
be produced using the procedures
prescribed. [S,S]-Ethylene diamine
disuccinic acid also was studied in
several primary eye irritation, primary
skin irritation, and dermal sensitization
studies. In two primary eye irritation
studies, two primary skin irritation
studies and a 24–hour repeat
application patch test, the substance
was considered a non-irritant. In a
dermal sensitization study and a human
repeat insult patch test, the substance
was found not to be a dermal sensitizer.
2. Genotoxicty. [S,S]-Ethylene
diamine disuccinic acid was shown not
to be genotoxic in a battery of standard
short-term studies. In a bacterial
mutation assay, it was concluded that,
when tested at dose levels up to 5,000
µg/plate of histidine dependent
auxotrophic mutants of Salmonella
typhimurium in water, [S,S]-ethylene
diamine disuccinic acid was not
mutagenic. In a Salmonella/mammalian
(Ames test) and Escherichia coli WP2
mutagenesis assay, [S,S]-ethylene
diamine disuccinic acid was tested
using tester strains TA98, TA100,
TA1535, TA1537, TA1538, WP2 uvrA
(pHM101), and WP2 (pHM101) in the
presence and absence of Aroclorinduced rat liver microsomal enzymes
at a maximum dose of 5,000 µg per plate
and was found not to cause a positive
response. Further, [S,S]-ethylene
diamine disuccinic acid was tested in a
L5178Y TK+/- mouse lymphoma
mutagenesis assay in the absence and
presence of aroclor induced rat liver S9, using doses of 4,028 to 2,765 µg/mL
in the initial assay and 5,028 to 2,765
µg/mL in the confirmatory assay, and
was found to be negative in both the
absence and presence of exogenous
metabolic activation. In an in vitro
cytogenetics assay with Chinese hamster
ovary (CHO) cells, in both definitive and
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confirmatory assays, the test system was
exposed to dose levels of 79, 157, 313,
625, 1,250, 2,500, and 5,000 µg/mL for
6 hours with a 12–hour recovery period
in the absence and presence of an S-9
reaction mixture. In addition, the test
system was exposed to 5, 10, 20, 40, 79,
157, 313, 625, and 1,250 µg/mL
continuously for 42 hours in the
absence of a S-9 reaction mixture. In the
definitive assay, survival at the highest
dose level was scored 82% in the nonactivated 6–hour treatment study, 70%
in the non-activated 18–hour treatment
study, 38% in the non-activated 42–
hour study, and 84% in the S-9
activated study. The three highest doses
with 200 scorable metaphase cells, i.e.,
313, 625, and 1,250 µg/mL in the 6–hour
non-activated study, 157, 313, and 625
µg/mL in the 6–hour activated study,
and 5, 10, and 20 µg/mL in the 42–hour
non-activated study, were selected for
microscopic analysis. The test article
did not induce a significant increase in
structural chromosome aberrations in
either the absence or presence of S-9
activation, regardless of the treatment
condition or harvest time (p≥0.025,
Fisher’s exact test). However, in the
non-activated 18–hour treatment study,
there were no scorable metaphase cells
in any of the test article dose groups. In
addition, there was a statistically
significant increase in numerical
aberrations in the non-activated 42–
hour study at 20 µg/mL (p<0.025,
Fisher’s exact test). There was also a
statistically significant dose response in
numerical aberrations in the nonactivated 42–hour study (p<0.05,
Cochran-Armitage test). In the
confirmatory assay, survival at the
highest dose level scored was 78% in
the non-activated 6–hour treatment
study, 77% in the non-activated 18–
hour study, 29% in the non-activated
42–hour treatment study, and 109% in
the S-9 activated study. The three
highest doses with 200 scorable
metaphase cells, i.e., 157, 313, and 625
µg/mL in the 6–hour treatment study,
313, 625, and 1,250 µg/mL in the 18–
hour non-activated study, and 10, 20,
and 40 µg/mL in the non-activated 42–
hour study, were selected for
microscopic analysis. The test article
did not induce a significant increase in
structural or numerical chromosome
aberrations in either the absence or
presence of S-9 activation in the 6–hour
or 18–hour treatment studies (p≥0.025,
Fisher’s exact test). There was a
statistically significant increase in
structural chromosome aberrations at
the 40 µg/mL dose level in the nonactivated 42–hour study (p<0.025,
Fisher’s exact test) and a statistically
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significant dose response (p<0.05,
Cochran-Armitage test). This increase in
the percentage of structural
chromosome aberrations in this dose
was within the acceptable range of the
historical control values, and therefore
this increase was not viewed as being
biologically relevant. Last, in an in vivo
cytogenetic assay in rats, male and
female Sprague-Dawley rats were
treated with [S,S]-ethylene diamine
disuccinic acid by single-dose gavage
administration of 200, 670, or 2,000 mg/
kg bwt. The percentage of structurally
damaged first division metaphase cells
was not significantly increased in the
test-article-treated groups, regardless of
sex, dose, or sacrifice time (p≤0.025,
Fisher’s exact test). The percentage of
numerically changed second division
metaphase cells was not significantly
increased in the test-article-treated
groups, regardless of sex, dose, or
sacrifice time (p>0.025, Fisher’s exact
test). It was concluded that [S,S]ethylene diamine disuccinic acid was
negative in the in vivo cryogenic assay
in rats.
3. Reproductive and developmental
toxicity. Two range-finding
developmental toxicity studies, two
developmental toxicity studies and one
plasma mineral level study were
conducted with rats. In the first rangefinding study, mated Charles River CRl:
CD VAF/Plus female rats were
administered 2,000, 8,000, 16,000,
24,000, and 40,000 parts per million of
the test substance in the diet on
gestation days 6 through 15. Maternal
toxicity resulted at the 16,000 ppm level
and higher, as evidenced by two test
article-related deaths at the highest dose
level, test article-related emaciation, soft
stool, decreased defacation and no stool,
and inhibited bodyweight gain, body
weight loss, and dose-related decreases
in food consumption when compared
with the control group. Developmental
toxicity was evidenced at 16,000 ppm
by reduced gravid uterine weight and at
doses of 24,000 ppm and above by
increases in post-implantation loss
when compared with the controls, and
a concomitant decrease in the numbers
of live fetuses. Developmental toxicity
also was evidenced from the fetuses
found to be severely malformed in the
24,000 ppm group. Based on the results
of this study, dosage levels of 0, 2,000,
8,000, and 16,000 ppm were selected by
the sponsors for the definitive
developmental toxicity study. In the
second range-finding study, mated
Charles River Crl:CD VAF/Plus female
rats were administered dosage levels of
the test article of 0, 50, 200, 400, 600,
and 1,000 mg/kg/day by gavage on
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gestation days 6 through 15. There were
no significant observations of maternal
toxicity at any dosage level. No
indication of developmental toxicity
was observed at the dose levels tested.
The study’s conclusion was the dose
levels evaluated produced no apparent
maternal or developmental toxicity that
was test article related. In the first
developmental toxicity study, mated
Charles River Crl:CD VAF/Plus female
rats were administered dosage levels of
2,000, 8,000, and 16,000 ppm of the test
substance in their diet on gestation days
6 through 15. Maternal toxicity was
evidenced at the high-dose level by
body weight and food consumption
inhibition as compared with the control
group. Blood zinc levels were decreased
in all treated groups, and iron and
copper levels were reduced in the highdose treated dams. Developmental
toxicity was indicated by a statistically
significant increase in post-implantation
losses at the high-dose level. Postimplantation losses at the high-dose
appeared to selectively affect the sex
ratio and, as a consequence, the
percentage of live male fetuses was
reduced while the percentage of live
female fetuses was increased.
Developmental toxicity also was
indicated for the high-dose group by
reduced fetal body weights.
Administration of the test article
resulted in teratogenicity in the majority
of fetuses and litters at a concentration
of 16,000 ppm. Fetuses from this group
were observed with singular or multiple
external, visceral and/or skeletal
malformations and developmental
variations. All major organ systems and
skeletal structures were affected. The
developmental period affected covers
the entire dose administration period;
therefore, the results of the study
indicate the test article is a nonselective teratogen capable of producing
a variety of malformations and
developmental changes. A depletion of
one or more metals in the blood, most
likely zinc, may be correlated with these
changes. In conclusion, the no observed
adverse effect level (NOAEL) for the test
substance when administered orally via
the diet to the mated rats was 8,000 ppm
with regard to maternal toxicity and
developmental toxicity. In the second
developmental toxicity study, the test
substance was administered to mated
Charles River Crl:CD VAF/Plus female
rats by oral gavage at dose levels of 0,
50, 400, and 1,000 mg/kg/day on
gestation days 6 through 15. Maternal
toxicity was indicated at the 1,000 mg/
kg/day dose level by a significant
reduction in mean carcass weights, a
significant reduction in food
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consumption, and an increased
incidence of clinical observations;
therefore, the NOAEL was considered to
be 400 mg/kg/day. Developmental
toxicity was not indicated at any dose
level evaluated, and the NOAEL with
respect to developmental toxicity was
considered greater than 1,000 mg/kg/
day. The plasma mineral levels in
pregnant rats were evaluated. In this
study, mated Charles River Crd:CD
VAF/Plus female rats were used to
determine the effect of the test
substance on plasma levels of zinc, iron
and copper in pregnant rats. Dose levels
of 50, 400, and 1,000 mg/kg/day were
administered by gavage as a single daily
dose on gestation days 6 through 15 at
a volume of 10.0 mL/kg. This resulted
in maternal toxicity at the 1,000 mg/kg/
day dose level, as indicated by soft stool
and reduced (non-statistically
significant) weight gain during the
treatment period. Treatment also
resulted in a dose-dependant,
statistically significant reduction in zinc
plasma levels for all dose groups at both
the 2 and 4 hour-time points, as
compared with the control group, and a
statistically significant dose-dependant
reduction in plasma copper levels in all
treated groups at 4 hours and at the two
highest dose levels at 2 hours. Plasma
levels of iron fluctuated in all treated
groups at both the 2 and 4 hour-time
points, as compared with the control
group, and these changes were not
considered due to treatment with the
test article. Oral administration of the
test article at dosages of 50, 400, and
1,000 mg/kg/day during gestation days 6
to 15 resulted in a dose-dependant
reduction in plasma zinc and copper in
samples obtained 2 and 4 hours after the
last dose on gestation day 15. Plasma
iron levels were reduced in the 50 and
400 mg/kg/day groups in a dosedependant fashion, as compared with
the control group, from samples
obtained at 2 and 4 hours following the
last dose on gestation day 15. This trend
was not observed at the 1,000 mg/kg/
day dosage, and there was no treatmentrelated effect on plasma iron levels at
this dose level. Administration of the
test article during the period of gestation
days 6 to 15 effectively lowered the
plasma levels of zinc and copper in a
dose-related fashion. There was no
dose-related effect in plasma iron levels
attributable to administration of the test
article.
4. Subchronic toxicity. Several shortterm studies were conducted using male
and female rats. In a 14–day oral feeding
study, one control and four dose groups
of male and female Wistar rats were
administered 0, 50, 500, 2,500, and
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5,000 mg/kg/bwt/day of the test
substance. In Group 5, the highest dose
group, one male was found dead on day
9 of treatment. In groups 1, 2, 3, and 4,
no deaths occurred. Test article related
clinical signs of reaction to treatment
with the test substance were noted in
Group 5 before death or sacrifice; ruffled
fur, diarrhea, emaciation, hunched
posture, and sedation were noted. In
Group 4, ruffled fur, diarrhea,
emaciation and hunched posture were
noted in both male and female animals
at the end of the first week and during
the second week. No clinical signs or
symptoms of ill health were noted in the
animals of Groups 1, 2, or 3. In a second
14–day oral feeding study with SFRbred male Wistar rats administered dose
levels of 0, 750, 1,000, and 1,250 mg/kg/
bwt/day, all animals survived until
scheduled necropsy, and no test article
related clinical signs were evident in
any animal. The mean food
consumption, body weight development
and relative food consumption were
unaffected by the test article. Based on
the results of this study, the no observed
effects level (NOEL) was considered to
be above 1,250 mg/kg/bwt/day. In a sub
chronic 13–week oral (feeding) toxicity
study, male and female SPF-bred Wistar
rats were fed nominal dose levels of the
test substance of 0, 50, 300, 700, and
1,000 mg/kg/bwt/day. Based on the
results, the NOEL of the test substance
was considered to be 300 mg/kg/bwt/
day. A mineral balance 28–day oral
toxicity (feeding) study using male rats
fed dose levels of the test substance of
0, 50, 150, 300, and 400 mg/kg/bwt/day
was conducted. Up to and including the
highest dose level, there were no test
article-related death or sign of reaction
to treatment. Food and water
consumption were not affected by
treatment with the test article. The
clinical laboratory data, opthalmoscopic
examination as well as the recording of
organ weights gave no indication of test
article related effects. At macroscopic
and microscopic examinations, no
treatment-related histopathologic
alterations in any of the organs or
tissues examined were noted. There
were no statistically significant changes
in body weight or body weight gain.
However, there was a trend towards a
decreased body weight and body weight
gain as the dose increased. The
increased urinary output of minerals
(Cu, Zn, Mg) was considered to be test
article-related. This increase in urinary
output was compensated by a decrease
in fecal elimination of the respective
minerals. There was no effect on total
mineral output relative to control
values. Tissue mineral (Cu, Zn, Mg)
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15:11 Jan 18, 2005
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levels were not affected in the sternum,
femur or liver. In the kidneys there was
a statistically significant decrease in
tissue Zn levels for two test groups. The
lack of a dose-response effect did not
allow for a definitive statement, but in
consideration of the effects of treatment
on Zn elimination, a test article-related
effect was not ruled out.
5. Chronic toxicity. [S,S]-ethylene
diamine disuccinic acid and its
metabolites are not structurally related
to a recognized carcinogen, and the
weight-of-the-evidence from the
reported genotoxicity and subchronic
toxicity studies indicates that [S,S]ethylene diamine disuccinic acid is not
mutagenic and does not produce a
morphologic effect in any organ that
could lead to neoplastic change.
6. Animal metabolism. The
absorption, distribution and elimination
of [S,S]-ethylene diamine disuccinic
acid were evaluated in three studies. In
the first study, succinate-14C(U)-[S,S]ethylene diamine disuccinic acid
sodium salt at 2,106 mg/kg was
administered to male Wistar rats by oral
(gavage) dosing. This resulted in
increased levels of radioactivity in bone
marrow over the first 24 hours followed
by biphasic elimination. The identity of
the radioactivity in tissues was not
determined. The mean peak bone
marrow radioactivity level was 37 µg
[S,S]-ethylene diamine disuccinic acid
sodium salt equivalents/g (ppm) at the
24–hour time point. Bone marrow
radioactivity levels declined thereafter
to 10 ppm at the end of the 72–hour
study period. Results of this study
demonstrate that bone marrow is
exposed to [S,S]-ethylene diamine
disuccinic acid and/or its metabolites
following oral (gavage) dosing under
conditions similar to those employed in
in vivo cytogenics studies. In the second
study, female Wistar rats were dosed
orally (gavage) with succinate-14C-(U)S,S-[S,S]-ethylene diamine disuccinic
acid sodium salt at 2053 mg/kg. This
resulted in elevated levels of
radioactivity in bone marrow during the
72–hour study period. The identity of
the radioactivity in tissues was not
determined. The highest mean bone
marrow radioactivity level was 14 µg
[S,S]-ethylene diamine disuccinic acid
sodium salt equivalents/g (ppm) at the
24–hour time point. Bone marrow
radioactivity declined slowly thereafter
to 5 ppm at the end of the 72–hour
period. Results of this study
demonstrate that bone marrow is
exposed to [S,S]-ethylene diamine
disuccinic acid and/or its metabolites
following oral (gavage) dosing under
conditions similar to those employed in
in vivo cytogenics studies. In the third
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Sfmt 4703
3031
study, groups of male and female Wistar
rats were administered 14C-[S,S]-[S,S]ethylene diamine disuccinic acid
sodium salt by oral gavage and dermal
application. Target dosing for the groups
varied between 10.0 ± 0.3 uCi/rat and
18.6 ± 0.5 uCi/rat. After oral
administration of 14C-[S,S]-[S,S]ethylene diamine disuccinic acid
sodium salt, radioactivity was rapidly
eliminated, mainly via the feces. Based
on the recovery of radioactivity in the
urine, expired air and tissues, the oral
absorption was less than approximately
5% of the dose in both gender groups.
Based on the radioactivity recoveries in
the excreta and the residue tissue
content, approximately 11.1% of the
applied dermal dose of 14C-[S,S]-[S,S]ethylene diamine disuccinic acid
sodium salt was absorbed by males and
5.18% was absorbed by females. During
dermal exposure of 14C-[S,S]-[S,S]ethylene diamine disuccinic acid
sodium salt, the amount of radioactivity
eliminated in the excreta of both gender
groups was less than 9% of the dose.
There was an apparent gender effect in
the amount of absorbed radioactivity
eliminated in the excreta for urine only.
There was no statistically significant
gender effect in the oral or dermal
absorption of radioactivity on the basis
of the radioactivity recoveries in the
excreta and tissue. The overall recovery
of radioactivity after oral administration
of 14C-[S,S]-[S,S]-ethylene diamine
disuccinic acid sodium salt was 84.4 ±
1.52% (males) and 89.5 ± (females) and
after dermal application was 59.1 ±
8.03% (males) and 62.8 ± 18.6%
(females) of the dose. There was no
statistically-significant difference in the
radioactivity recoveries between the
male and female animals after both
routes of administration.
7. Metabolite toxicology. [S,S]Ethylene diamine disuccinic acid occurs
in nature and is a siderophore produced
by the Actinomycetes, Amycolatopis
japonica sp. nov. (Ref. 2) and
Amycolatopsis orientalis (Ref 3). [S,S]Ethylene diamine disuccinic acid is
rapidly and completely mineralized
(Ref. 4). The degradation pathway of
[S,S]-ethylene diamine disuccinic acid
is not fully understood. However, the
catabolism of [S,S]-ethylene diamine
disuccinic acid was initiated by carbonnitrogen lyase catalysing the nonhydrolytic cleavage of the C-N bond
between the ethlenediamine part of the
molecule and one of the succinyl
residues without any collectors being
required. The reaction led to the
formation of fumarate and AEAA [N-(2aminoethyl) aspartic acid]. The further
degradation of AEAA remains still to be
E:\FR\FM\19JAN1.SGM
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unraveled. To date, one can merely
speculate that, catalysed by DH
(dehydrogenase) or a MO
(monooxygenase), the C-N bond
between the succinyl residue and the
ethylene diamine part of the molecule is
split, or that an aspartyl residue is
removed by the cleavage of a C-N bond
within the ethylenediamine part of
AEAA. (Ref. 5). [S,S]-ethylene diamine
disuccinic acid and related [S,S]
homologues comply with
internationally accepted criteria for
ready biodegradability of chemicals
‘‘ostensibly because the metabolic
products of the biodegradation are
naturally occurring biochemicals such
as succinic acid’’ (Ref. 6).
8. Endocrine disruption. [S,S]Ethylene diamine disuccinic acid does
not belong to a class of chemicals
known or suspected of having adverse
effects on the endocrine system. There
is no evidence that [S,S]-ethylene
diamine disuccinic acid had any effect
on endocrine function in the
developmental or reproduction studies.
C. Aggregate Exposure
1. Dietary exposure. As a minor
formulation component, and given its
rapid and complete mineralization,
there is no reasonable expectation that
[S,S]-ethylene diamine disuccinic acid
will appear in the diet.
i. Food. As a minor formulation
component, and given its rapid and
complete mineralization, there is no
reasonable expectation that [S,S]ethylene diamine disuccinic acid will
appear in the diet.
ii. Drinking water. As a minor
formulation component, and given its
rapid and complete mineralization,
there is no reasonable expectation that
[S,S]-ethylene diamine disuccinic acid
will appear in water.
2. Non-dietary exposure. Non-dietary
exposures to [S,S]-ethylene diamine
disuccinic acid will be both
occupational and residential.
Occupational exposures include those
to applicators and handlers of pesticides
containing this substance. However,
precautionary measures prescribed by
the labels of pesticide products
containing this substance will minimize
these exposures. Also, [S,S]-ethylene
diamine disuccinic acid is used in the
U.S. in the metal treatment industry as
a chelating agent. However, the
precautionary measures prescribed by
the product’s material safety data sheet
will minimize exposure to workers in
this industry. [S,S]-Ethylene diamine
disuccinic acid also is used in the U.S.
in hair dye products as a chelating agent
to stabilize the peroxide bleach portion.
Exposure to [S,S]-ethylene diamine
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15:11 Jan 18, 2005
Jkt 205001
disuccinic acid in these residential
products should be minimal because the
products are used for limited periods
and [S,S]-ethylene diamine disuccinic
acid is used in minor amounts in the
products.
D. Cumulative Effects
The potential for [S,S]-ethylene
diamine disuccinic acid and other
substances that have a common
mechanism of toxicity has been
considered. [S,S]-Ethylene diamine
disuccinic acid is a naturally occurring
substance produced by certain common
bacteria, and it is rapidly and
completely mineralized in the
environment. There is no reliable
information to indicate that toxic effects
produced by [S,S]-ethylene diamine
disuccinic acid would be cumulative
with those of any other chemicals,
including another pesticide. Therefore,
the Associated Octel Corporation,
Limited believes that it is appropriate to
consider only the potential risks of
[S,S]-ethylene diamine disuccinic acid
in an aggregate risk assessment.
E. Safety Determination
1. U.S. population. As presented
previously, the exposures of the U.S.
general population to [S,S]-ethylene
diamine disuccinic acid are low, few
hazards are presented by [S,S]-ethylene
diamine disuccinic acid, and the risks
are minimal. Use of [S,S]-ethylene
diamine disuccinic acid as a minor
component of pesticide formulations
applied to growing crops would not
contribute significantly to the level of
[S,S]-ethylene diamine disuccinic acid
found naturally in the environment and
to which man is exposed. Further, there
is adequate information to show that
any toxicological concern raised by the
potential contribution of [S,S]-ethylene
diamine disuccinic acid to growing
crops is minimal. Occupational
exposure to [S,S]-ethylene diamine
disuccinic acid is expected to be well
controlled and limited if worker-safety
procedures are routinely practiced.
Residential exposure also should be
minimal, because of the low levels of
[S,S]-ethylene diamine disuccinic acid
contained in hair dyes and the
infrequent, intermittent use of these
products.
2. Infants and children. The complete
toxicological data base, including the
developmental toxicity studies, was
considered in assessing the potential for
additional sensitivity of infants and
children to residues of [S,S]-ethylene
diamine disuccinic acid. The
developmental toxicity studies did
indicate an increased sensitivity of rats
to in-utero exposure to [S,S]-ethylene
PO 00000
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Fmt 4703
Sfmt 4703
diamine disuccinic acid. However, this
increased sensitivity appeared at very
high dose levels which also caused
maternal toxicity, and these levels are
not expected to appear in or on growing
crops, because [S,S]-ethylene diamine
disuccinic acid is a minor component of
pesticide formulations and it will
rapidly and completely mineralize after
application.
F. International Tolerances
There are no known international
tolerances for residues of [S,S]-ethylene
diamine disuccinic acid in food or
animal feed.
G. References
1. Brady, N. C. 1990. The Nature and
Properties of Soils. MacMillan
Publishing Company. New York, New
York.
2. Goodfellow, M., A. B. Brown, J. Cai,
J. Chun and M. D. Collins. 1997.
Amycolatopsis Japonicum sp. nov., and
Actinomycete producing (S,S)-N,N’ethylene diamine disuccinic acid.
System. Appl. Microbiol. 20,78-84.
3. Zwicker, N., U. Theobald, H.
Zahner and H-D Fielder. 1997.
Optimization of fermantation conditions
for the production of ethylene diamine
disuccinic acid by Amycolatopsis
orientalis. Journal of Industrial
Microbiology & Biotechnology. 19, 280285.
4. Schowanek D., T. C. J. Feijtel, C. M.
Perkins F.A. Hartman, T. W. Federle, R.
J. Larson. 1997. Biodegradation of [S,S]
[R,R] and mixed stereoisomers of
ethylene diamine disuccinic acid
(EDDS), a transition metal chelator.
Chemosphere, Vol. 34, No. 11, pp 23752391.
5. Bucheli-Witschel, M. and T. Egli.
2001. Environmental fate and
microdegradation of
aminopolycarboxylic acids. FEMS
Microbiology Reviews. 25pp 69-106.
6. Whitburn, J. S., S. D. Wilkinson and
D. R. Williams. 1999. Chemical
speciation of ethylene diamine-N, N′disuccinic acid (EDDS) and its metal
complexes in solution. Chemical
Speciation and Bioavailability. 11(3) pp
85-93.
[FR Doc. 05–824 Filed 1–18–05; 8:45 am]
BILLING CODE 6560–50–S
ENVIRONMENTAL PROTECTION
AGENCY
[FRL–7861–9]
Carolina Steel Drum Superfund Site;
Notice of Proposed Settlement
AGENCY:
Environmental Protection
Agency.
E:\FR\FM\19JAN1.SGM
19JAN1
Agencies
[Federal Register Volume 70, Number 12 (Wednesday, January 19, 2005)]
[Notices]
[Pages 3026-3032]
From the Federal Register Online via the Government Printing Office [www.gpo.gov]
[FR Doc No: 05-824]
-----------------------------------------------------------------------
ENVIRONMENTAL PROTECTION AGENCY
[OPP-2004-0297; FRL-7690-5]
[S,S]-Ethylene diamine disuccinic acid; Notice of Filing a
Pesticide Petition to Establish a Tolerance for a Certain Pesticide
Chemical in or on Food
AGENCY: Environmental Protection Agency (EPA).
[[Page 3027]]
ACTION: Notice.
-----------------------------------------------------------------------
SUMMARY: This notice announces the initial filing of a pesticide
petition proposing the establishment of regulations for residues of a
certain pesticide chemical in or on various food commodities.
DATES: Comments, identified by docket identification (ID) number OPP-
2004-0297, must be received on or before February 18, 2005.
ADDRESSES: Comments may be submitted electronically, by mail, or
through hand delivery/courier. Follow the detailed instructions as
provided in Unit I. of the SUPPLEMENTARY INFORMATION.
FOR FURTHER INFORMATION CONTACT: Bipin Gandhi, Registration Division
(7505C), Office of Pesticide Programs, Environmental Protection Agency,
1200 Pennsylvania Ave., NW., Washington, DC 20460-0001; telephone
number: (703) 308-8380; e-mail address: gandhi.bipin@epa.gov.
SUPPLEMENTARY INFORMATION:
I. General Information
A. Does this Action Apply to Me?
You may be potentially affected by this action if you are an
agricultural producer, food manufacturer, or pesticide manufacturer.
Potentially affected entities may include, but are not limited to:
Crop production (NAICS 111)
Animal production (NAICS 112)
Food manufacturing (NAICS 311)
Pesticide manufacturing (NAICS 32532)
This listing is not intended to be exhaustive, but rather provides
a guide for readers regarding entities likely to be affected by this
action. Other types of entities not listed in this unit could also be
affected. The North American Industrial Classification System (NAICS)
codes have been provided to assist you and others in determining
whether this action might apply to certain entities. If you have any
questions regarding the applicability of this action to a particular
entity, consult the person listed under FOR FURTHER INFORMATION
CONTACT.
B. How Can I Get Copies of this Document and Other Related Information?
1. Docket. EPA has established an official public docket for this
action under docket ID number OPP-2004-0297. The official public docket
consists of the documents specifically referenced in this action, any
public comments received, and other information related to this action.
Although a part of the official docket, the public docket does not
include Confidential Business Information (CBI) or other information
whose disclosure is restricted by statute. The official public docket
is the collection of materials that is available for public viewing at
the Public Information and Records Integrity Branch (PIRIB), Rm. 119,
Crystal Mall 2, 1801 S. Bell St., Arlington, VA. This docket
facility is open from 8:30 a.m. to 4 p.m., Monday through Friday,
excluding legal holidays. The docket telephone number is (703) 305-
5805.
2. Electronic access. You may access this Federal Register document
electronically through the EPA Internet under the ``Federal Register''
listings at https://www.epa.gov/fedrgstr/.
An electronic version of the public docket is available through
EPA's electronic public docket and comment system, EPA Dockets. You may
use EPA Dockets at https://www.epa.gov/edocket/ to submit or view public
comments, access the index listing of the contents of the official
public docket, and to access those documents in the public docket that
are available electronically. Although not all docket materials may be
available electronically, you may still access any of the publicly
available docket materials through the docket facility identified in
Unit I.B.1. Once in the system, select ``search,'' then key in the
appropriate docket ID number.
Certain types of information will not be placed in the EPA Dockets.
Information claimed as CBI and other information whose disclosure is
restricted by statute, which is not included in the official public
docket, will not be available for public viewing in EPA's electronic
public docket. EPA's policy is that copyrighted material will not be
placed in EPA's electronic public docket but will be available only in
printed, paper form in the official public docket. To the extent
feasible, publicly available docket materials will be made available in
EPA's electronic public docket. When a document is selected from the
index list in EPA Dockets, the system will identify whether the
document is available for viewing in EPA's electronic public docket.
Although not all docket materials may be available electronically, you
may still access any of the publicly available docket materials through
the docket facility identified in Unit I.B. EPA intends to work towards
providing electronic access to all of the publicly available docket
materials through EPA's electronic public docket.
For public commenters, it is important to note that EPA's policy is
that public comments, whether submitted electronically or in paper,
will be made available for public viewing in EPA's electronic public
docket as EPA receives them and without change, unless the comment
contains copyrighted material, CBI, or other information whose
disclosure is restricted by statute. When EPA identifies a comment
containing copyrighted material, EPA will provide a reference to that
material in the version of the comment that is placed in EPA's
electronic public docket. The entire printed comment, including the
copyrighted material, will be available in the public docket.
Public comments submitted on computer disks that are mailed or
delivered to the docket will be transferred to EPA's electronic public
docket. Public comments that are mailed or delivered to the docket will
be scanned and placed in EPA's electronic public docket. Where
practical, physical objects will be photographed, and the photograph
will be placed in EPA's electronic public docket along with a brief
description written by the docket staff.
C. How and to Whom Do I Submit Comments?
You may submit comments electronically, by mail, or through hand
delivery/courier. To ensure proper receipt by EPA, identify the
appropriate docket ID number in the subject line on the first page of
your comment. Please ensure that your comments are submitted within the
specified comment period. Comments received after the close of the
comment period will be marked ``late.'' EPA is not required to consider
these late comments. If you wish to submit CBI or information that is
otherwise protected by statute, please follow the instructions in Unit
I.D. Do not use EPA Dockets or e-mail to submit CBI or information
protected by statute.
1. Electronically. If you submit an electronic comment as
prescribed in this unit, EPA recommends that you include your name,
mailing address, and an e-mail address or other contact information in
the body of your comment. Also include this contact information on the
outside of any disk or CD ROM you submit, and in any cover letter
accompanying the disk or CD ROM. This ensures that you can be
identified as the submitter of the comment and allows EPA to contact
you in case EPA cannot read your comment due to technical difficulties
or needs further information on the substance of your comment. EPA's
policy is that EPA will not edit your comment, and any identifying or
contact information provided in the body of a comment will
[[Page 3028]]
be included as part of the comment that is placed in the official
public docket, and made available in EPA's electronic public docket. If
EPA cannot read your comment due to technical difficulties and cannot
contact you for clarification, EPA may not be able to consider your
comment.
i. EPA Dockets. Your use of EPA's electronic public docket to
submit comments to EPA electronically is EPA's preferred method for
receiving comments. Go directly to EPA Dockets at https://www.epa.gov/
edocket/, and follow the online instructions for submitting comments.
Once in the system, select ``search,'' and then key in docket ID number
OPP-2004-0297. The system is an ``anonymous access'' system, which
means EPA will not know your identity, e-mail address, or other contact
information unless you provide it in the body of your comment.
ii. E-mail. Comments may be sent by e-mail to opp-docket@epa.gov,
Attention: Docket ID Number OPP-2004-0297. In contrast to EPA's
electronic public docket, EPA's e-mail system is not an ``anonymous
access'' system. If you send an e-mail comment directly to the docket
without going through EPA's electronic public docket, EPA's e-mail
system automatically captures your e-mail address. E-mail addresses
that are automatically captured by EPA's e-mail system are included as
part of the comment that is placed in the official public docket, and
made available in EPA's electronic public docket.
iii. Disk or CD ROM. You may submit comments on a disk or CD ROM
that you mail to the mailing address identified in Unit I.C.2. These
electronic submissions will be accepted in WordPerfect or ASCII file
format. Avoid the use of special characters and any form of encryption.
2. By mail. Send your comments to: Public Information and Records
Integrity Branch (PIRIB) (7502C), Office of Pesticide Programs (OPP),
Environmental Protection Agency, 1200 Pennsylvania Ave., NW.,
Washington, DC 20460-0001, Attention: Docket ID Number OPP-2004-0297.
3. By hand delivery or courier. Deliver your comments to: Public
Information and Records Integrity Branch (PIRIB), Office of Pesticide
Programs (OPP), Environmental Protection Agency, Rm. 119, Crystal Mall
2, 1801 S. Bell St., Arlington, VA, Attention: Docket ID
Number OPP-2004-0297. Such deliveries are only accepted during the
docket's normal hours of operation as identified in Unit I.B.1.
D. How Should I Submit CBI to the Agency?
Do not submit information that you consider to be CBI
electronically through EPA's electronic public docket or by e-mail. You
may claim information that you submit to EPA as CBI by marking any part
or all of that information as CBI (if you submit CBI on disk or CD ROM,
mark the outside of the disk or CD ROM as CBI and then identify
electronically within the disk or CD ROM the specific information that
is CBI). Information so marked will not be disclosed except in
accordance with procedures set forth in 40 CFR part 2.
In addition to one complete version of the comment that includes
any information claimed as CBI, a copy of the comment that does not
contain the information claimed as CBI must be submitted for inclusion
in the public docket and EPA's electronic public docket. If you submit
the copy that does not contain CBI on disk or CD ROM, mark the outside
of the disk or CD ROM clearly that it does not contain CBI. Information
not marked as CBI will be included in the public docket and EPA's
electronic public docket without prior notice. If you have any
questions about CBI or the procedures for claiming CBI, please consult
the person listed under FOR FURTHER INFORMATION CONTACT.
E. What Should I Consider as I Prepare My Comments for EPA?
You may find the following suggestions helpful for preparing your
comments:
1. Explain your views as clearly as possible.
2. Describe any assumptions that you used.
3. Provide copies of any technical information and/or data you used
that support your views.
4. If you estimate potential burden or costs, explain how you
arrived at the estimate that you provide.
5. Provide specific examples to illustrate your concerns.
6. Make sure to submit your comments by the deadline in this
notice.
7. To ensure proper receipt by EPA, be sure to identify the docket
ID number assigned to this action in the subject line on the first page
of your response. You may also provide the name, date, and Federal
Register citation.
II. What Action is the Agency Taking?
EPA has received a pesticide petition as follows proposing the
establishment and/or amendment of regulations for residues of a certain
pesticide chemical in or on various food commodities under section 408
of the Federal Food, Drug, and Cosmetic Act (FFDCA), 21 U.S.C. 346a.
EPA has determined that this petition contains data or information
regarding the elements set forth in FFDCA section 408(d)(2); however,
EPA has not fully evaluated the sufficiency of the submitted data at
this time or whether the data support granting of the petition.
Additional data may be needed before EPA rules on the petition.
List of Subjects
Environmental protection, Agricultural commodities, Feed additives,
Food additives, Pesticides and pests, Reporting and recordkeeping
requirements.
Dated: December 29, 2004.
Betty Shackleford,
Acting Director, Registration Division, Office of Pesticide Programs.
Summary of Petition
The petitioner summary of the pesticide petition is printed below
as required by FFDCA section 408(d)(3). The summary of the petition was
prepared by the petitioner and represents the view of the petitioner.
The summary may have been edited by EPA if the terminology used was
unclear, the summary contained extraneous material, or the summary
unintentionally made the reader conclude that the findings reflected
EPA's position and not the position of the petitioner. The petition
summary announces the availability of a description of the analytical
methods available to EPA for the detection and measurement of the
pesticide chemical residues or an explanation of why no such method is
needed.
The Associated Octel Company, Limited
PP 4E6818
EPA has received a pesticide petition (4E6818) from The Associated
Octel Company, Limited, P.O. Box 17, Oil Sites Road, Ellesmere Port,
South Wirral L65 4HF, United Kingdom proposing, pursuant to section
408(d) of the FFDCA, 21 U.S.C. 346a(d), to amend 40 CFR part 180 to
establish an exemption from the requirement of a tolerance for [S,S]-
ethylene diamine disuccinic acid, CAS Reg. No. 20846-91-7. EPA has
determined that the petition contains data or information regarding the
elements set forth in section 408(d)(2) of the FFDCA; however, EPA has
not fully evaluated the sufficiency of the submitted data at this time
or whether the data support granting of the petition.
[[Page 3029]]
Additional data may be needed before EPA rules on the petition.
A. Residue Chemistry
1. Plant metabolism. [S,S]-Ethylene diamine disuccinic acid is a
chelating agent that is used as a vehicle to deliver micronutrients
essential for healthy and rapid growth, such as iron and cobalt, to
plants. It is unknown whether or not plants would uptake [S,S]-ethylene
diamine disuccinic acid that might leach into the soil when applied as
a minor component of pesticide formulations. However, organic chelating
agents are not absorbed normally by growing plants. It appears that the
primary role the chelate plays is to hold the metallic cations near the
root surface until direct absorption of the free cation can take place.
Once the micronutrient cations are inside the plant, other organic
chelates (such as citrates) may be carriers of these cations to
different parts of the plant (Ref. 1). Therefore, it is unlikely that
[S,S]-ethylene diamine disuccinic acid would accumulate within plant
tissue through its application to the soil as a minor component of
pesticide formulations.
2. Analytical method. An analytical method has not been proposed
because [S,S]-ethylene diamine disuccinic acid residues harmful to
plants and animals are highly unlikely to occur when it is applied as
part of the proposed pesticide formulation and according to that
formulation's label directions for use.
3. Magnitude of residues. A waiver of the residue data has been
requested because [S,S]-ethylene diamine disuccinic acid is produced by
actinomycetes, Amycolatopis japonica sp. nov. (Ref. 2) and
Amycolatopsis orientalis (Ref. 3), which are naturally occurring
bacteria, degrades rapidly and is completely mineralized in the soil,
will have limited accessibility to plants in the proposed use pattern,
and exhibits low mammalian toxicity. [S,S]-Ethylene diamine disuccinic
acid is a siderophore produced by actinomycetes, and it functions
symbiotically with plants to assist in the transport of soil metals to
plant rootlets. The use of [S,S]-ethylene diamine disuccinic acid,
therefore, does not constitute the addition of a foreign material to
the soil; rather, it is a compound that soil microorganisms and plants
already encounter. Natural mechanisms already exist for the degradation
and/or utilization of [S,S]-ethylene diamine disuccinic acid in the
soil/plant microsystem. Moreover, organic chelates are not absorbed
normally by growing plants, and residues are not expected in plants.
B. Toxicological Profile
1. Acute toxicity. The acute toxicity of [S,S]-ethylene diamine
disuccinic acid was studied in several studies using male and female
rats via the oral, dermal, and inhalation routes. In two acute oral
toxicity studies, the lethal dose (LD)50 for both males and
females was established at >2,700 milligrams/kilogram body weight (mg/
kg bwt) and >2,000 mg/kg bwt, respectively, which were the highest dose
levels tested. For the two acute dermal toxicity studies, the
LD50 for both males and females was established at >2,640
mg/kg bwt and > 2,000 mg/kg bwt, respectively, which were the highest
dose levels tested. For the acute inhalation study, the lethal
concentration (LC)50 was established at >1.49 milligrams/
liter (mg/L), which was the highest concentration that could be
produced using the procedures prescribed. [S,S]-Ethylene diamine
disuccinic acid also was studied in several primary eye irritation,
primary skin irritation, and dermal sensitization studies. In two
primary eye irritation studies, two primary skin irritation studies and
a 24-hour repeat application patch test, the substance was considered a
non-irritant. In a dermal sensitization study and a human repeat insult
patch test, the substance was found not to be a dermal sensitizer.
2. Genotoxicty. [S,S]-Ethylene diamine disuccinic acid was shown
not to be genotoxic in a battery of standard short-term studies. In a
bacterial mutation assay, it was concluded that, when tested at dose
levels up to 5,000 [mu]g/plate of histidine dependent auxotrophic
mutants of Salmonella typhimurium in water, [S,S]-ethylene diamine
disuccinic acid was not mutagenic. In a Salmonella/mammalian (Ames
test) and Escherichia coli WP2 mutagenesis assay, [S,S]-ethylene
diamine disuccinic acid was tested using tester strains TA98, TA100,
TA1535, TA1537, TA1538, WP2 uvrA (pHM101), and WP2 (pHM101) in the
presence and absence of Aroclor-induced rat liver microsomal enzymes at
a maximum dose of 5,000 [mu]g per plate and was found not to cause a
positive response. Further, [S,S]-ethylene diamine disuccinic acid was
tested in a L5178Y TK+/- mouse lymphoma mutagenesis assay in the
absence and presence of aroclor induced rat liver S-9, using doses of
4,028 to 2,765 [mu]g/mL in the initial assay and 5,028 to 2,765 [mu]g/
mL in the confirmatory assay, and was found to be negative in both the
absence and presence of exogenous metabolic activation. In an in vitro
cytogenetics assay with Chinese hamster ovary (CHO) cells, in both
definitive and confirmatory assays, the test system was exposed to dose
levels of 79, 157, 313, 625, 1,250, 2,500, and 5,000 [mu]g/mL for 6
hours with a 12-hour recovery period in the absence and presence of an
S-9 reaction mixture. In addition, the test system was exposed to 5,
10, 20, 40, 79, 157, 313, 625, and 1,250 [mu]g/mL continuously for 42
hours in the absence of a S-9 reaction mixture. In the definitive
assay, survival at the highest dose level was scored 82% in the non-
activated 6-hour treatment study, 70% in the non-activated 18-hour
treatment study, 38% in the non-activated 42-hour study, and 84% in the
S-9 activated study. The three highest doses with 200 scorable
metaphase cells, i.e., 313, 625, and 1,250 [mu]g/mL in the 6-hour non-
activated study, 157, 313, and 625 [mu]g/mL in the 6-hour activated
study, and 5, 10, and 20 [mu]g/mL in the 42-hour non-activated study,
were selected for microscopic analysis. The test article did not induce
a significant increase in structural chromosome aberrations in either
the absence or presence of S-9 activation, regardless of the treatment
condition or harvest time (p>=0.025, Fisher's exact test). However, in
the non-activated 18-hour treatment study, there were no scorable
metaphase cells in any of the test article dose groups. In addition,
there was a statistically significant increase in numerical aberrations
in the non-activated 42-hour study at 20 [mu]g/mL (p<0.025, Fisher's
exact test). There was also a statistically significant dose response
in numerical aberrations in the non-activated 42-hour study (p<0.05,
Cochran-Armitage test). In the confirmatory assay, survival at the
highest dose level scored was 78% in the non-activated 6-hour treatment
study, 77% in the non-activated 18-hour study, 29% in the non-activated
42-hour treatment study, and 109% in the S-9 activated study. The three
highest doses with 200 scorable metaphase cells, i.e., 157, 313, and
625 [mu]g/mL in the 6-hour treatment study, 313, 625, and 1,250 [mu]g/
mL in the 18-hour non-activated study, and 10, 20, and 40 [mu]g/mL in
the non-activated 42-hour study, were selected for microscopic
analysis. The test article did not induce a significant increase in
structural or numerical chromosome aberrations in either the absence or
presence of S-9 activation in the 6-hour or 18-hour treatment studies
(p>=0.025, Fisher's exact test). There was a statistically significant
increase in structural chromosome aberrations at the 40 [mu]g/mL dose
level in the non-activated 42-hour study (p<0.025, Fisher's exact test)
and a statistically
[[Page 3030]]
significant dose response (p<0.05, Cochran-Armitage test). This
increase in the percentage of structural chromosome aberrations in this
dose was within the acceptable range of the historical control values,
and therefore this increase was not viewed as being biologically
relevant. Last, in an in vivo cytogenetic assay in rats, male and
female Sprague-Dawley rats were treated with [S,S]-ethylene diamine
disuccinic acid by single-dose gavage administration of 200, 670, or
2,000 mg/kg bwt. The percentage of structurally damaged first division
metaphase cells was not significantly increased in the test-article-
treated groups, regardless of sex, dose, or sacrifice time (p<=0.025,
Fisher's exact test). The percentage of numerically changed second
division metaphase cells was not significantly increased in the test-
article-treated groups, regardless of sex, dose, or sacrifice time
(p>0.025, Fisher's exact test). It was concluded that [S,S]-ethylene
diamine disuccinic acid was negative in the in vivo cryogenic assay in
rats.
3. Reproductive and developmental toxicity. Two range-finding
developmental toxicity studies, two developmental toxicity studies and
one plasma mineral level study were conducted with rats. In the first
range-finding study, mated Charles River CRl: CD VAF/Plus female rats
were administered 2,000, 8,000, 16,000, 24,000, and 40,000 parts per
million of the test substance in the diet on gestation days 6 through
15. Maternal toxicity resulted at the 16,000 ppm level and higher, as
evidenced by two test article-related deaths at the highest dose level,
test article-related emaciation, soft stool, decreased defacation and
no stool, and inhibited bodyweight gain, body weight loss, and dose-
related decreases in food consumption when compared with the control
group. Developmental toxicity was evidenced at 16,000 ppm by reduced
gravid uterine weight and at doses of 24,000 ppm and above by increases
in post-implantation loss when compared with the controls, and a
concomitant decrease in the numbers of live fetuses. Developmental
toxicity also was evidenced from the fetuses found to be severely
malformed in the 24,000 ppm group. Based on the results of this study,
dosage levels of 0, 2,000, 8,000, and 16,000 ppm were selected by the
sponsors for the definitive developmental toxicity study. In the second
range-finding study, mated Charles River Crl:CD VAF/Plus female rats
were administered dosage levels of the test article of 0, 50, 200, 400,
600, and 1,000 mg/kg/day by gavage on gestation days 6 through 15.
There were no significant observations of maternal toxicity at any
dosage level. No indication of developmental toxicity was observed at
the dose levels tested. The study's conclusion was the dose levels
evaluated produced no apparent maternal or developmental toxicity that
was test article related. In the first developmental toxicity study,
mated Charles River Crl:CD VAF/Plus female rats were administered
dosage levels of 2,000, 8,000, and 16,000 ppm of the test substance in
their diet on gestation days 6 through 15. Maternal toxicity was
evidenced at the high-dose level by body weight and food consumption
inhibition as compared with the control group. Blood zinc levels were
decreased in all treated groups, and iron and copper levels were
reduced in the high-dose treated dams. Developmental toxicity was
indicated by a statistically significant increase in post-implantation
losses at the high-dose level. Post-implantation losses at the high-
dose appeared to selectively affect the sex ratio and, as a
consequence, the percentage of live male fetuses was reduced while the
percentage of live female fetuses was increased. Developmental toxicity
also was indicated for the high-dose group by reduced fetal body
weights. Administration of the test article resulted in teratogenicity
in the majority of fetuses and litters at a concentration of 16,000
ppm. Fetuses from this group were observed with singular or multiple
external, visceral and/or skeletal malformations and developmental
variations. All major organ systems and skeletal structures were
affected. The developmental period affected covers the entire dose
administration period; therefore, the results of the study indicate the
test article is a non-selective teratogen capable of producing a
variety of malformations and developmental changes. A depletion of one
or more metals in the blood, most likely zinc, may be correlated with
these changes. In conclusion, the no observed adverse effect level
(NOAEL) for the test substance when administered orally via the diet to
the mated rats was 8,000 ppm with regard to maternal toxicity and
developmental toxicity. In the second developmental toxicity study, the
test substance was administered to mated Charles River Crl:CD VAF/Plus
female rats by oral gavage at dose levels of 0, 50, 400, and 1,000 mg/
kg/day on gestation days 6 through 15. Maternal toxicity was indicated
at the 1,000 mg/kg/day dose level by a significant reduction in mean
carcass weights, a significant reduction in food consumption, and an
increased incidence of clinical observations; therefore, the NOAEL was
considered to be 400 mg/kg/day. Developmental toxicity was not
indicated at any dose level evaluated, and the NOAEL with respect to
developmental toxicity was considered greater than 1,000 mg/kg/day. The
plasma mineral levels in pregnant rats were evaluated. In this study,
mated Charles River Crd:CD VAF/Plus female rats were used to determine
the effect of the test substance on plasma levels of zinc, iron and
copper in pregnant rats. Dose levels of 50, 400, and 1,000 mg/kg/day
were administered by gavage as a single daily dose on gestation days 6
through 15 at a volume of 10.0 mL/kg. This resulted in maternal
toxicity at the 1,000 mg/kg/day dose level, as indicated by soft stool
and reduced (non-statistically significant) weight gain during the
treatment period. Treatment also resulted in a dose-dependant,
statistically significant reduction in zinc plasma levels for all dose
groups at both the 2 and 4 hour-time points, as compared with the
control group, and a statistically significant dose-dependant reduction
in plasma copper levels in all treated groups at 4 hours and at the two
highest dose levels at 2 hours. Plasma levels of iron fluctuated in all
treated groups at both the 2 and 4 hour-time points, as compared with
the control group, and these changes were not considered due to
treatment with the test article. Oral administration of the test
article at dosages of 50, 400, and 1,000 mg/kg/day during gestation
days 6 to 15 resulted in a dose-dependant reduction in plasma zinc and
copper in samples obtained 2 and 4 hours after the last dose on
gestation day 15. Plasma iron levels were reduced in the 50 and 400 mg/
kg/day groups in a dose-dependant fashion, as compared with the control
group, from samples obtained at 2 and 4 hours following the last dose
on gestation day 15. This trend was not observed at the 1,000 mg/kg/day
dosage, and there was no treatment-related effect on plasma iron levels
at this dose level. Administration of the test article during the
period of gestation days 6 to 15 effectively lowered the plasma levels
of zinc and copper in a dose-related fashion. There was no dose-related
effect in plasma iron levels attributable to administration of the test
article.
4. Subchronic toxicity. Several short-term studies were conducted
using male and female rats. In a 14-day oral feeding study, one control
and four dose groups of male and female Wistar rats were administered
0, 50, 500, 2,500, and
[[Page 3031]]
5,000 mg/kg/bwt/day of the test substance. In Group 5, the highest dose
group, one male was found dead on day 9 of treatment. In groups 1, 2,
3, and 4, no deaths occurred. Test article related clinical signs of
reaction to treatment with the test substance were noted in Group 5
before death or sacrifice; ruffled fur, diarrhea, emaciation, hunched
posture, and sedation were noted. In Group 4, ruffled fur, diarrhea,
emaciation and hunched posture were noted in both male and female
animals at the end of the first week and during the second week. No
clinical signs or symptoms of ill health were noted in the animals of
Groups 1, 2, or 3. In a second 14-day oral feeding study with SFR-bred
male Wistar rats administered dose levels of 0, 750, 1,000, and 1,250
mg/kg/bwt/day, all animals survived until scheduled necropsy, and no
test article related clinical signs were evident in any animal. The
mean food consumption, body weight development and relative food
consumption were unaffected by the test article. Based on the results
of this study, the no observed effects level (NOEL) was considered to
be above 1,250 mg/kg/bwt/day. In a sub chronic 13-week oral (feeding)
toxicity study, male and female SPF-bred Wistar rats were fed nominal
dose levels of the test substance of 0, 50, 300, 700, and 1,000 mg/kg/
bwt/day. Based on the results, the NOEL of the test substance was
considered to be 300 mg/kg/bwt/day. A mineral balance 28-day oral
toxicity (feeding) study using male rats fed dose levels of the test
substance of 0, 50, 150, 300, and 400 mg/kg/bwt/day was conducted. Up
to and including the highest dose level, there were no test article-
related death or sign of reaction to treatment. Food and water
consumption were not affected by treatment with the test article. The
clinical laboratory data, opthalmoscopic examination as well as the
recording of organ weights gave no indication of test article related
effects. At macroscopic and microscopic examinations, no treatment-
related histopathologic alterations in any of the organs or tissues
examined were noted. There were no statistically significant changes in
body weight or body weight gain. However, there was a trend towards a
decreased body weight and body weight gain as the dose increased. The
increased urinary output of minerals (Cu, Zn, Mg) was considered to be
test article-related. This increase in urinary output was compensated
by a decrease in fecal elimination of the respective minerals. There
was no effect on total mineral output relative to control values.
Tissue mineral (Cu, Zn, Mg) levels were not affected in the sternum,
femur or liver. In the kidneys there was a statistically significant
decrease in tissue Zn levels for two test groups. The lack of a dose-
response effect did not allow for a definitive statement, but in
consideration of the effects of treatment on Zn elimination, a test
article-related effect was not ruled out.
5. Chronic toxicity. [S,S]-ethylene diamine disuccinic acid and its
metabolites are not structurally related to a recognized carcinogen,
and the weight-of-the-evidence from the reported genotoxicity and
subchronic toxicity studies indicates that [S,S]-ethylene diamine
disuccinic acid is not mutagenic and does not produce a morphologic
effect in any organ that could lead to neoplastic change.
6. Animal metabolism. The absorption, distribution and elimination
of [S,S]-ethylene diamine disuccinic acid were evaluated in three
studies. In the first study, succinate-14C(U)-[S,S]-ethylene diamine
disuccinic acid sodium salt at 2,106 mg/kg was administered to male
Wistar rats by oral (gavage) dosing. This resulted in increased levels
of radioactivity in bone marrow over the first 24 hours followed by
biphasic elimination. The identity of the radioactivity in tissues was
not determined. The mean peak bone marrow radioactivity level was 37
[mu]g [S,S]-ethylene diamine disuccinic acid sodium salt equivalents/g
(ppm) at the 24-hour time point. Bone marrow radioactivity levels
declined thereafter to 10 ppm at the end of the 72-hour study period.
Results of this study demonstrate that bone marrow is exposed to [S,S]-
ethylene diamine disuccinic acid and/or its metabolites following oral
(gavage) dosing under conditions similar to those employed in in vivo
cytogenics studies. In the second study, female Wistar rats were dosed
orally (gavage) with succinate-14C-(U)-S,S-[S,S]-ethylene diamine
disuccinic acid sodium salt at 2053 mg/kg. This resulted in elevated
levels of radioactivity in bone marrow during the 72-hour study period.
The identity of the radioactivity in tissues was not determined. The
highest mean bone marrow radioactivity level was 14 [mu]g [S,S]-
ethylene diamine disuccinic acid sodium salt equivalents/g (ppm) at the
24-hour time point. Bone marrow radioactivity declined slowly
thereafter to 5 ppm at the end of the 72-hour period. Results of this
study demonstrate that bone marrow is exposed to [S,S]-ethylene diamine
disuccinic acid and/or its metabolites following oral (gavage) dosing
under conditions similar to those employed in in vivo cytogenics
studies. In the third study, groups of male and female Wistar rats were
administered 14C-[S,S]-[S,S]-ethylene diamine disuccinic acid sodium
salt by oral gavage and dermal application. Target dosing for the
groups varied between 10.0 0.3 uCi/rat and 18.6 0.5 uCi/rat. After oral administration of 14C-[S,S]-[S,S]-
ethylene diamine disuccinic acid sodium salt, radioactivity was rapidly
eliminated, mainly via the feces. Based on the recovery of
radioactivity in the urine, expired air and tissues, the oral
absorption was less than approximately 5% of the dose in both gender
groups. Based on the radioactivity recoveries in the excreta and the
residue tissue content, approximately 11.1% of the applied dermal dose
of 14C-[S,S]-[S,S]-ethylene diamine disuccinic acid sodium salt was
absorbed by males and 5.18% was absorbed by females. During dermal
exposure of 14C-[S,S]-[S,S]-ethylene diamine disuccinic acid sodium
salt, the amount of radioactivity eliminated in the excreta of both
gender groups was less than 9% of the dose. There was an apparent
gender effect in the amount of absorbed radioactivity eliminated in the
excreta for urine only. There was no statistically significant gender
effect in the oral or dermal absorption of radioactivity on the basis
of the radioactivity recoveries in the excreta and tissue. The overall
recovery of radioactivity after oral administration of 14C-[S,S]-[S,S]-
ethylene diamine disuccinic acid sodium salt was 84.4
1.52% (males) and 89.5 (females) and after dermal
application was 59.1 8.03% (males) and 62.8
18.6% (females) of the dose. There was no statistically-significant
difference in the radioactivity recoveries between the male and female
animals after both routes of administration.
7. Metabolite toxicology. [S,S]-Ethylene diamine disuccinic acid
occurs in nature and is a siderophore produced by the Actinomycetes,
Amycolatopis japonica sp. nov. (Ref. 2) and Amycolatopsis orientalis
(Ref 3). [S,S]-Ethylene diamine disuccinic acid is rapidly and
completely mineralized (Ref. 4). The degradation pathway of [S,S]-
ethylene diamine disuccinic acid is not fully understood. However, the
catabolism of [S,S]-ethylene diamine disuccinic acid was initiated by
carbon-nitrogen lyase catalysing the non-hydrolytic cleavage of the C-N
bond between the ethlenediamine part of the molecule and one of the
succinyl residues without any collectors being required. The reaction
led to the formation of fumarate and AEAA [N-(2-aminoethyl) aspartic
acid]. The further degradation of AEAA remains still to be
[[Page 3032]]
unraveled. To date, one can merely speculate that, catalysed by DH
(dehydrogenase) or a MO (monooxygenase), the C-N bond between the
succinyl residue and the ethylene diamine part of the molecule is
split, or that an aspartyl residue is removed by the cleavage of a C-N
bond within the ethylenediamine part of AEAA. (Ref. 5). [S,S]-ethylene
diamine disuccinic acid and related [S,S] homologues comply with
internationally accepted criteria for ready biodegradability of
chemicals ``ostensibly because the metabolic products of the
biodegradation are naturally occurring biochemicals such as succinic
acid'' (Ref. 6).
8. Endocrine disruption. [S,S]-Ethylene diamine disuccinic acid
does not belong to a class of chemicals known or suspected of having
adverse effects on the endocrine system. There is no evidence that
[S,S]-ethylene diamine disuccinic acid had any effect on endocrine
function in the developmental or reproduction studies.
C. Aggregate Exposure
1. Dietary exposure. As a minor formulation component, and given
its rapid and complete mineralization, there is no reasonable
expectation that [S,S]-ethylene diamine disuccinic acid will appear in
the diet.
i. Food. As a minor formulation component, and given its rapid and
complete mineralization, there is no reasonable expectation that [S,S]-
ethylene diamine disuccinic acid will appear in the diet.
ii. Drinking water. As a minor formulation component, and given its
rapid and complete mineralization, there is no reasonable expectation
that [S,S]-ethylene diamine disuccinic acid will appear in water.
2. Non-dietary exposure. Non-dietary exposures to [S,S]-ethylene
diamine disuccinic acid will be both occupational and residential.
Occupational exposures include those to applicators and handlers of
pesticides containing this substance. However, precautionary measures
prescribed by the labels of pesticide products containing this
substance will minimize these exposures. Also, [S,S]-ethylene diamine
disuccinic acid is used in the U.S. in the metal treatment industry as
a chelating agent. However, the precautionary measures prescribed by
the product's material safety data sheet will minimize exposure to
workers in this industry. [S,S]-Ethylene diamine disuccinic acid also
is used in the U.S. in hair dye products as a chelating agent to
stabilize the peroxide bleach portion. Exposure to [S,S]-ethylene
diamine disuccinic acid in these residential products should be minimal
because the products are used for limited periods and [S,S]-ethylene
diamine disuccinic acid is used in minor amounts in the products.
D. Cumulative Effects
The potential for [S,S]-ethylene diamine disuccinic acid and other
substances that have a common mechanism of toxicity has been
considered. [S,S]-Ethylene diamine disuccinic acid is a naturally
occurring substance produced by certain common bacteria, and it is
rapidly and completely mineralized in the environment. There is no
reliable information to indicate that toxic effects produced by [S,S]-
ethylene diamine disuccinic acid would be cumulative with those of any
other chemicals, including another pesticide. Therefore, the Associated
Octel Corporation, Limited believes that it is appropriate to consider
only the potential risks of [S,S]-ethylene diamine disuccinic acid in
an aggregate risk assessment.
E. Safety Determination
1. U.S. population. As presented previously, the exposures of the
U.S. general population to [S,S]-ethylene diamine disuccinic acid are
low, few hazards are presented by [S,S]-ethylene diamine disuccinic
acid, and the risks are minimal. Use of [S,S]-ethylene diamine
disuccinic acid as a minor component of pesticide formulations applied
to growing crops would not contribute significantly to the level of
[S,S]-ethylene diamine disuccinic acid found naturally in the
environment and to which man is exposed. Further, there is adequate
information to show that any toxicological concern raised by the
potential contribution of [S,S]-ethylene diamine disuccinic acid to
growing crops is minimal. Occupational exposure to [S,S]-ethylene
diamine disuccinic acid is expected to be well controlled and limited
if worker-safety procedures are routinely practiced. Residential
exposure also should be minimal, because of the low levels of [S,S]-
ethylene diamine disuccinic acid contained in hair dyes and the
infrequent, intermittent use of these products.
2. Infants and children. The complete toxicological data base,
including the developmental toxicity studies, was considered in
assessing the potential for additional sensitivity of infants and
children to residues of [S,S]-ethylene diamine disuccinic acid. The
developmental toxicity studies did indicate an increased sensitivity of
rats to in-utero exposure to [S,S]-ethylene diamine disuccinic acid.
However, this increased sensitivity appeared at very high dose levels
which also caused maternal toxicity, and these levels are not expected
to appear in or on growing crops, because [S,S]-ethylene diamine
disuccinic acid is a minor component of pesticide formulations and it
will rapidly and completely mineralize after application.
F. International Tolerances
There are no known international tolerances for residues of [S,S]-
ethylene diamine disuccinic acid in food or animal feed.
G. References
1. Brady, N. C. 1990. The Nature and Properties of Soils. MacMillan
Publishing Company. New York, New York.
2. Goodfellow, M., A. B. Brown, J. Cai, J. Chun and M. D. Collins.
1997. Amycolatopsis Japonicum sp. nov., and Actinomycete producing
(S,S)-N,N'-ethylene diamine disuccinic acid. System. Appl. Microbiol.
20,78-84.
3. Zwicker, N., U. Theobald, H. Zahner and H-D Fielder. 1997.
Optimization of fermantation conditions for the production of ethylene
diamine disuccinic acid by Amycolatopsis orientalis. Journal of
Industrial Microbiology & Biotechnology. 19, 280-285.
4. Schowanek D., T. C. J. Feijtel, C. M. Perkins F.A. Hartman, T.
W. Federle, R. J. Larson. 1997. Biodegradation of [S,S] [R,R] and mixed
stereoisomers of ethylene diamine disuccinic acid (EDDS), a transition
metal chelator. Chemosphere, Vol. 34, No. 11, pp 2375-2391.
5. Bucheli-Witschel, M. and T. Egli. 2001. Environmental fate and
microdegradation of aminopolycarboxylic acids. FEMS Microbiology
Reviews. 25pp 69-106.
6. Whitburn, J. S., S. D. Wilkinson and D. R. Williams. 1999.
Chemical speciation of ethylene diamine-N, N'-disuccinic acid (EDDS)
and its metal complexes in solution. Chemical Speciation and
Bioavailability. 11(3) pp 85-93.
[FR Doc. 05-824 Filed 1-18-05; 8:45 am]
BILLING CODE 6560-50-S